Optics (physics.optics)

Abstract: Flatbands play an important role in correlated quantum matter and have novel applications in photonic lattices. Synthetic magnetic fields and destructive interference in lattices are traditionally used to obtain flatbands. However, such methods can only obtain a few flatbands with most bands remaining dispersive. Here we realize all-band-flat photonic lattices of an arbitrary size by precisely controlling the coupling strengths between lattice sites to mimic those in Fock-state lattices. This allows us to go beyond the perturbative regime of strain engineering and group all eigenmodes in flatbands, which simultaneously achieves high band flatness and large usable bandwidth. We map out the distribution of each flatband in the lattices and selectively excite the eigenmodes with different chiralities. Our method paves a new way in controlling band structure and topology of photonic lattices.

Abstract: Chiral molecules show differences in their chemical and optical properties due to different spatial arrangements of the atoms in the two enantiomers. A common way to optically differentiate them is to detect the disparity in the absorption of light by the two enantiomers, i.e. the absorption circular dichroism (CD). However, the CD of typical molecules is very small, limiting the sensitivity of chiroptical analysis based on CD. Cavity ring-down spectroscopy (CRDS) is a well-known ultrasensitive absorption spectroscopic method for low-absorbing gas-phase samples because the multiple reflections of light in the cavity greatly increase the absorption path. By inserting a prism into the cavity, the optical mode undergoes total internal reflection (TIR) at the prism surface and the evanescent wave (EW) enables the absorption detection of condensed-phase samples within a very thin layer near the prism surface, called EW-CRDS. Here, we propose an ultrasensitive chiral absorption spectroscopy platform using a dielectric metasurface-assisted EW-CRDS. We theoretically show that, upon linearly polarized and oblique incidence, the metasurface exhibits minimum scattering and absorption loss, introduces negligible polarization change, and locally converts the linearly polarized light into near fields with finite optical chirality, enabling CD detection with EW-CRDS that only works with linearly polarized light. We evaluate the ring-down time in the presence of chiral molecules and determine the sensitivity of the cavity as a function of total absorption from the molecules. The findings open the avenue for an ultrasensitive thin film detection of the chiral molecules using the CRDS techniques.

Abstract: Fluorescence molecular tomography (FMT) is a promising modality for non-invasive imaging of internal fluorescence agents in biological tissues especially in small animal models, with applications in diagnosis, therapy, and drug design. In this paper, we present a new fluorescent reconstruction algorithm that combines time-resolved fluorescence imaging data with photon-counting micro-CT (PCMCT) images to estimate the quantum yield and lifetime of fluorescent markers in a mouse model. By incorporating PCMCT images, a permissible region of interest of fluorescence yield and lifetime can be roughly estimated as prior knowledge, reducing the number of unknown variables in the inverse problem and improving image reconstruction stability. Our numerical simulation results demonstrate the accuracy and stability of this method in the presence of data noise, with an average relative error of 18% in fluorescent yield and lifetime reconstruction.

Abstract: Single epitaxial quantum dots (QDs) are a leading technology for quantum light generation, particularly when embedded in photonic devices that enhance their emission. However, coupling this emission into a desirable optical channel, like a single mode fiber, is often challenging. Direct laser writing (DLW) enables the fabrication of three-dimensional sub-micron features out of photoresist, supporting micro- and nano- scale devices that can address this challenge. In this study, we use DLW to directly waveguide-couple epitaxially-grown InAs/GaAs QDs by fabricating 1 $\mu$m diameter polymer nanowires (PNWs) in contact with the GaAs substrate housing the QDs. The PNWs are high index contrast cylindrical waveguides perpendicular to the GaAs device layer, which couple the emission from an underlying QD to the HE$_{11}$ mode of the PNW, enhancing the collection efficiency to a single-mode fiber. PNW fabrication does not alter the QD device layer (e.g., via etching), making PNWs well suited for augmenting existing photonic geometries that enhance QD emission. We study PNWs as standalone devices and in conjunction with metallic nanorings -- an already-established geometry for increasing vertical extraction of light from embedded QDs. Since PNWs are fabricated on substrates that abosorb and reflect at the DLW exposure wavelength, we report methods to mitigate standing wave reflections and heat, which otherwise prevent PNW fabrication. We observe a factor of ($3.0 \pm 0.7)\times$ improvement in a nanoring system with a PNW compared to the same system without a PNW, in line with numerical results, highlighting a PNW's ability to waveguide QD emission and increase collection efficiency simultaneously. These results demonstrate a new approach in which DLW can provide additional functionality for quantum emitter photonics, in a manner compatible with existing top-down fabrication approaches.