Optics (physics.optics)

Abstract: Classical electrodynamics describes the optical response of macroscopic systems, where the boundaries between materials is treated as infinitesimally thin. However, due to the quantum nature of electrons, interfaces acquires a finite thickness. To include non-classical surface effects in the framework of Maxwell's equations, surface-response functions can be introduced, also known as Feibelman $d$-parameters. Surface response impacts systems with strong field localization at interfaces, which is encountered in noble metal nanoparticles supporting surface plasmon polaritons. However, studying surface response is challenging as it necessitates sub-nanometer control of geometric features, e.g. the gap size in a dimer antenna, while minimizing uncertainties in morphology. In contrast, electrical gating is convenient since the static screening charges are confined exclusively to the surface, which alleviates the need for precise control over the morphology. Here, we study the perturbation of Feibelman $d$-parameters by direct electric charging of a single plasmonic nanoresonator and investigate the resulting changes of the resonance in experiment and theory. The measured change of the resonance frequency matches the theory by assuming a perturbation of the tangential surface current. However, we also observe an unforeseen narrowing in the resonance width when adding electrons to the surface of a plasmonic nanoresonator. These reduced losses cannot be explained by electron spill-out within the local-response approximation (LRA). Such an effect is likely caused by nonlocality and the anisotropy of the perturbed local permittivity. Our findings open up possibilities to reduce losses in plasmonic resonators and to develop ultrafast and extremely small electrically driven plasmonic modulators and metasurfaces by leveraging electrical control over non-classical surface effects.

Abstract: Spatiotemporal modulation offers a variety of opportunities for light manipulations. In this paper, we propose a way towards arbitrary transformation for pulses sequentially propagating within one waveguide in space via temporal waveguide coupling. The temporal waveguide coupling operation is achieved by spatiotemporally modulating the refractive index of the spatial waveguide with a traveling wave through segmented electrodes. We derive the temporal coupled-mode equations and discuss how systematic parameters affect the temporal coupling coefficients. We further demonstrated a temporal Mach-Zehnder interferometer and universal multiport interferometer, which enables arbitrary unitary transformation for pulses. We showcase a universal approach for transforming pulses among coupled temporal waveguides, which requires only one spatial waveguide under spatiotemporal modulation, and hence provide a flexible, compact, and highly compatible method for optical signal processing in time domain.

Abstract: Optical bistability is fundamental for all-optical switches, but typically requires high-Q cavities with micrometer sizes. Through boosting nonlinearity with photo-thermo-optical effects, we achieve bistability in a silicon Mie resonator with a volume size of 10-3 um3 and Q-factor < 10, both are record-low. Furthermore, bistable scattering naturally leads to large super-linear emission-excitation power dependence, which we applied to enhance optical resolution by more than 3 times. Our work paves the way toward nanoscale photonics computation and label-free semiconductor nano-inspection.

Abstract: Bound states in the continuum (BICs) theoretically have the ability to confine electromagnetic waves in limited regions with infinite radiative quality ($Q$) factors. However, in practical experiments, resonances can only exhibit finite $Q$ factors due to unwanted scattering losses caused by fabrication imperfections. Recently, it has been shown that ultrahigh-$Q$ guided-mode resonances (GMRs), which are robust to fabrication imperfections, can be realized by merging multiple BICs in momentum space. In this study, we analytically and numerically investigate the merging and band transition of accidental BICs in planar photonic lattices. Accidental BICs can merge at the edges of the second stop band, either with or without a symmetry-protected BIC. We show that as the thickness of the photonic lattice gradually increases, the merged state of BICs transitions from the upper to the lower band edge. Using coupled-mode analysis, we present the analytical merging thickness at which multiple accidental BICs merge at the second-order $\Gamma$ point. Our coupled-mode analysis could be beneficial for achieving ultrahigh-$Q$ GMRs in various photonic lattices composed of materials with different dielectric constants.

Abstract: A near-eye display device (NED) is a visual optical system that places a miniature display in front of the human eye to provide an immersive viewing experience. NEDs have been playing an irreplaceable role in both early military flight applications and today's civil and entertainment applications. In this paper, we propose an easy-to-machine design of a near-eye display based on surface relief grating waveguides, taking into account the experience of previous designs of near-eye displays, the superior performance of the design, and the accuracy level of existing grating processing. The design is designed to meet the requirements of large field of view and large outgoing pupil extension as much as possible. The design is insensitive to the incident angle and achieves a full-field field-of-view angle of 40{\deg}, an angular uniformity error of 20% for diffraction efficiency, and an average diffraction efficiency of 80% for the full field of view. Based on the design, the overall simulation of the optical path of the NED device is completed, and the illumination uniformity of the outgoing pupil expansion of the device is analyzed through simulation.

Abstract: A photonic crystal microcavity with the liquid crystal resonant layer tunable by heating has been implemented. The multiple vanishing resonant lines corresponding to optical bound states in the continuum are observed. The abrupt behaviour of the resonant linewidth near the vanishing point can be used for temperature sensing.

Abstract: Chirality is a concept that one object is not superimposable on its mirror image by translation and rotation. In particular, chiral plasmonics have been widely investigated due to the their excellent optical chiral properties, and have led to numerous applications such as optical polarizing element etc. In this study, we develop a model based on the concept of the interaction between harmonic oscillators to investigate and explain the optical chiral mechanisms of strongly coupled metal nanoparticles (MNPs). The chirality of the scattering, absorption, and photoluminescence spectra are carefully discussed in detail. The results show that the chirality of the system originates not only from the orientations of the MNPs, but also from the different eigen parameters between them. Specifically, the derived three factors contribute to the chirality: the symmetry, the coupling strength, and the coherent superposition of the emitted electric field. This work provides a deeper understanding on the chiral plasmonics and may guide relevant applications in theory.

Abstract: Imaging polarimetry based on dielectric metasurface is well-known for its ultra-compactness and high integration. However, previous works suffer from low energy efficiency, limited restrictions on choice of target polarization states, or inability to focus light. Here, by inverse design, we numerically demonstrate a multi-foci metalens-based polarimetry that can simultaneously separate and focus the four free-chosen elliptical polarization states at the wavelength of 10.6 \mu m. Such a full-stokes polarimetry features an average absolute efficiency up to 54.63%, and an average relative error as low as 0.00137%. This spatial-multiplexing-free full stokes polarimetry exceeds the theoretical maximum efficiency of traditional polarization-filtering counterparts, and resolves the restriction faced by the orthogonal polarization-multiplexed method.

Abstract: Interferometric scattering microscopy (iSCAT) can image the dynamics of nanometer-scale systems. The typical approach to analyzing interferometric images involves intensive processing, which discards data and limits the precision of measurements. We demonstrate an alternative approach: modeling the interferometric point spread function (iPSF) and fitting this model to data within a Bayesian framework. This approach yields best-fit parameters, including the particle's three-dimensional position and polarizability, as well as uncertainties and correlations between these parameters. Building on recent work, we develop a model that is parameterized for rapid fitting. The model is designed to work with Hamiltonian Monte Carlo techniques that leverage automatic differentiation. We validate this approach by fitting the model to interferometric images of colloidal nanoparticles. We apply the method to track a diffusing particle in three dimensions, to directly infer the diffusion coefficient of a nanoparticle without calculating a mean-square displacement, and to quantify the ejection of DNA from an individual lambda phage virus, demonstrating that the approach can be used to infer both static and dynamic properties of nanoscale systems.

Abstract: We demonstrate a technique that allows highly surface sensitive imaging of nanostructures on planar surfaces over large areas, providing a new avenue for research in materials science, especially for \textit{in situ} applications. The capabilities of hard X-ray grazing incidence ptychography combine aspects from imaging, reflectometry and grazing incidence small angle scattering in providing large field-of-view images with high resolution transverse to the beam, horizontally and along the surface normal. Thus, it yields data with resolutions approaching electron microscopy, in two dimensions, but over much larger areas and with a poorer resolution in the third spatial dimension, along the beam propagation direction. Similar to grazing incidence small angle X-ray scattering, this technique facilitates the characterization of nanostructures across statistically significant surface areas or volumes within potentially feasible time frames for \textit{in situ} experiments, while also providing spatial information.

Abstract: All-optical modulation yields the promise of high-speed information processing. In this frame, metasurfaces are rapidly gaining traction as ultrathin multifunctional platforms for light management. Among the featured functionalities, they enable light wavefront manipulation and, more recently, demonstrated the ability to perform light-by-light manipulation through nonlinear optical processes. Here, by employing a nonlinear periodic metasurface, we demonstrate all-optical routing of telecom photons upconverted to the visible range. This is achieved via the interference between two frequency-degenerate upconversion processes, namely third-harmonic and sum-frequency generation, stemming from the interaction of a pump pulse with its frequency-doubled replica. By tuning the relative phase and polarization between these two pump beams, and concurrently engineering the nonlinear emission of the individual elements of the metasurfaces (meta-atoms) along with its pitch, we route the upconverted signal among the diffraction orders of the metasurface with a modulation efficiency up to 90%. Thanks to the phase control and the ultrafast dynamics of the underlying nonlinear processes, free-space all-optical routing could be potentially performed at rates close to the employed optical frequencies divided by the quality factor of the optical resonances at play. Our approach adds a further twist to optical interferometry, which is a key-enabling technique in a wide range of applications, such as homodyne detection, radar interferometry, LiDAR technology, gravitational waves detection, and molecular photometry. In particular, the nonlinear character of light upconversion combined with phase sensitivity is extremely appealing for enhanced imaging and biosensing.

Abstract: This work compares two tomographic imaging technologies, time-domain full-field optical coherence tomography (FFOCT) working in reflection and optical transmission tomography (OTT), using a new optical setup that combines both. We show that, due to forward-scattering properties, the axial sectioning and contrast in OTT can be optimized by tuning illumination. The influence of sample scattering and thickness are discussed. We illustrate the comparison of the two methods in static (morphology) and dynamic (metabolic contrast) regimes using cell cultures, tissues and entire organisms emphasizing the advantages of both approaches.