Optics (physics.optics)

Abstract: Optical pulses propagating in multimode optical fibers are affected by linear disorder and nonlinearity, and experience chaotic exchange of power among modes. On the other hand, complex systems can attain steady states characterized by energy condensation into single as well multiple sub-systems. In this work, we study beam propagation in multimode optical fibers in the presence of linear random mode coupling and Kerr nonlinearity; both effects lead to a mode power redistribution at the fiber output. We use a new 3D mode decomposition method to obtain, with unprecedented accuracy, measurements of the modal distribution from long spans of graded-index fiber; we perform numerical simulations using a new model for the linear disorder; we introduce a weighted Bose-Einstein law and show that it is suitable for describing steady-state modal power distributions both in the linear and nonlinear regimes. We show that, at power levels intermediate between the linear and the soliton regimes, energy condensation is attained locally by the second, third and fourth modal groups, before global condensation to the fundamental mode is reached in the soliton regime. Our results extend the thermodynamic approach to multimode fibers to unexplored optical states, which acquire the characteristics of optical glass.

Abstract: Microresonators are micron-scale optical systems that confine light using total internal reflection. These optical systems have gained interest in the last two decades due to their compact sizes, unprecedented measurement capabilities, and widespread applications. The increasingly high finesse (or $Q$ factor) of such resonators means that nonlinear effects are unavoidable even for low power, making them attractive for nonlinear applications, including optical comb generation and second harmonic generation. In addition, light in these nonlinear resonators may exhibit chaotic behavior across wide parameter regions. Hence, it is necessary to understand how, where, and what types of such chaotic dynamics occur before they can be used in practical devices. We consider a pair of coupled differential equations that describes the interactions of two optical beams in a single-mode resonator with symmetric pumping. Recently, it was shown that this system exhibits a wide range of fascinating behaviors, including bistability, symmetry breaking, chaos, and self-switching oscillations. We employ here a dynamical system approach to identify, delimit, and explain the regions where such different behaviors can be observed. Specifically, we find that different kinds of self-switching oscillations are created via the collision of a pair of asymmetric periodic orbits or chaotic attractors at Shilnikov homoclinic bifurcations, which acts as a gluing bifurcation. We present a bifurcation diagram that shows how these global bifurcations are organized by a Belyakov transition point (where the stability of the homoclinic orbit changes). In this way, we map out distinct transitions to different chaotic switching behavior that should be expected from this optical device.

Abstract: Monolayer (1L) transition metal dichalcogenides (TMDC) are of strong interest in nanophotonics due to their narrow-band intense excitonic transitions persisting up to room temperature. When brought into resonance with surface plasmon polariton (SPP) excitations of a conductive medium opportunities for studying and engineering strong light-matter coupling arise. Here, we consider a most simple geometry, namely a planar stack composed of a thin silver film, an Al2O3 spacer and a monolayer of WS2. We perform total internal reflection ellipsometry which combines spectroscopic ellipsometry with the Kretschmann-Raether-type surface plasmon resonance configuration. The combined amplitude and phase response of the reflected light at varied angle of incidence proves that despite the atomic thinness of 1L-WS2, the strong coupling (SC) regime between A excitons and SPPs propagating in the thin Ag film is reached. The phasor representation of rho corroborates SC as rho undergoes a topology change indicated by the occurrence of a double point at the cross over from the weak to the strong coupling regime. Our findings are validated by both analytical transfer matrix method calculations and numerical Maxwell simulations. The findings open up new perspectives for applications in plasmonic modulators and sensors benefitting from the tunability of the optical properties of 1L-TMDCs by electric fields, electrostatic doping, light and the chemical environment.

Abstract: Phase retardation is a cornerstone of modern optics, yet, at mid-infrared (mid-IR) frequencies, it remains a major challenge due to the scarcity of simultaneously transparent and birefringent crystals. Most materials resonantly absorb due to lattice vibrations occurring at mid-IR frequencies, and natural birefringence is weak, calling for hundreds of microns to millimeters-thick phase retarders for sufficient polarization rotation. We demonstrate mid-IR phase retardation with flakes of $\alpha$-molybdenum trioxide ($\alpha$-MoO$_3$) that are more than ten times thinner than the operational wavelength, achieving 90 degrees polarization rotation within one micrometer of material. We report conversion ratios above 50% in reflection and transmission mode, and wavelength tunability by several micrometers. Our results showcase that exfoliated flakes of low-dimensional crystals can serve as a platform for mid-IR miniaturized integrated polarization control.

Abstract: Coupled nanolasers are of growing interest for on-chip optical computation and data transmission, which requires an understanding of how lasers interact to form complex systems. The non-Hermitian interaction between two coupled resonators, when excited selectively, can lead to parity-time symmetry, the formation of exceptional points, and subsequently spectral control and increased sensitivity. These investigations have been limited to pump energies close to the lasing threshold, and large or narrow-line lasers. Here, by programmable optical excitation we study two coupled nanolasers significantly above threshold, where mode instability plays an important role. We map the mode evolution around two exceptional points, and observe lasing gaps due to reversed pump dependence which compare well with nonlinear theory. Finally, the coupling can be exploited to control the lasing threshold and wavelength, and for frequency switching around the lasing gap. Controlled and integrated nanolasers constitutes a promising platform for future highly sensitive and programmable on-chip laser sources.

Abstract: In the past years, optical fluorescence microscopy (OFM) made steady progress towards increasing the localisation precision of fluorescent emitters in biological samples. The high precision achieved by these techniques has prompted new claims, whose rigorous validation is an outstanding problem. For this purpose, local estimation theory (LET) has emerged as the most used mathematical tool. We establish a novel multi-parameter estimation framework that captures the full complexity of single-emitter localisation in an OFM experiment. Our framework relies on the fact that there are other unknown parameters alongside the emitter's coordinates, such as the average number of photons emitted (brightness), that are correlated to the emitter position, and affect the localisation precision. The increasing complexity of a multi-parameter approach allows for a more accountable assessment of the precision. We showcase our method with MINFLUX microscopy, the OFM approach that nowadays generates images with the best resolution. Introducing the brightness as an unknown parameter, we shed light on features that remain obscure in the conventional approach: the precision can be increased only by increasing the brightness, (i.e., illumination power or exposition time), whereas decreasing the beam separation offers limited advantages. We demonstrate that the proposed framework is a solid and general method for the quantification of single-emitter localisation precision for any OFM approach on equal footing, evaluating the localization precision of stimulated emission depletion (STED) microscopy and making a comparison with MINFLUX microscopy.

Abstract: In this contribution, we develop a model based on classical electrodynamics that describes light extinction in the presence of arbitrary aerosols. We do this by combining aerosol and light-intensity measurements performed with the well-proven measuring systems ELPI+ and MIREX, respectively. The developed model is particularly simple and depends on only a few input parameters, namely on densities and refractive indices of the constituting aerosol particles. As proof of principle, the model is in first applications used to determine extinction coefficients as well as mass-specific extinction for an infrared light source with a peak wave length of ${\lambda} = 0.88\ {\mu}m$. In doing so, detailed studies concentrate on two aerosols exemplary for characteristic values of the input parameters: a non-absorbing paraffin aerosol in a bench-scale setup and soot from a flaming n-heptane fire in a room-scale setup (test fire TF5 according to standard EN54). As main results, we find numerical values for mass-specific extinction that are first of all different in the two considered cases. Moreover, obtained results differ in part more than a factor of three from literature values typically used in practical applications. Based on the developed model, we explicitly address and assess underlying reasons for the deviations found. Finally, we propose a simple way how future light-extinction studies can be performed comparatively easily by means of the ELPI+-system or measuring devices that work in a similar way.

Abstract: A simple technique for observing optically stimulated electron paramagnetic resonance (OSEPR) is proposed and investigated. The versatility and information content of the described technique is demonstrated by the example of the OSEPR spectra of systems that are unpopular for this type of spectroscopy: a crystal with rare-earth ions Nd$^{3+}$ and a doped semiconductor GaAs. In addition, the OSEPR spectrum of atomic cesium is presented, in which an optical nonlinearity is observed that makes it possible to estimate the Rabi frequency for the relevant optical transition. The effects observed in the described experiments (switching of peaks to dips, light-induced splitting of the OSEPR lines, and the appearance of a spectral feature at the double-Larmor frequency) are interpreted using the model proposed in the theoretical part of the work. The suggested interpretation shows the possibility of using the described OSEPR technique to estimate not only `magnetic' parameters of the model Hamiltonian (g-factors, spin relaxation times), but also the Rabi frequencies characterizing optical transitions.

Abstract: The ability to perform attosecond-pump attosecond-probe spectroscopy (APAPS) is a longstanding goal in ultrafast science. While first pioneering experiments demonstrated the feasibility of APAPS, the low repetition rates (10-120 Hz) and the large footprints of existing setups have so far hindered the widespread exploitation of APAPS. Here we demonstrate two-color APAPS using a commercial laser system at 1 kHz, straightforward post-compression in a hollow-core fiber and a compact high-harmonic generation (HHG) setup. The latter enables the generation of intense extreme-ultraviolet (XUV) pulses by using an out-of-focus HHG geometry and by exploiting a transient blueshift of the driving laser in the HHG medium. Near-isolated attosecond pulses are generated, as demonstrated by one-color and two-color XUV-pump XUV-probe experiments. Our concept allows selective pumping and probing on extremely short timescales and permits investigations of fundamental processes that are not accessible by other pump-probe techniques.

Abstract: X-ray Fluorescence Ghost Imaging (XRF-GI) was recently demonstrated for x-ray lab sources. It has the potential to reduce acquisition time and deposited dose by choosing their trade-off with spatial resolution, while alleviating the focusing constraints of the probing beam. Here, we demonstrate the realization of synchrotron-based XRF-GI: We present both an adapted experimental setup and its corresponding required computational technique to process the data. This not only extends the above-mentioned advantages to synchrotron XRF imaging, it also presents new possibilities for developing strategies to improve precision in nano-scale imaging measurements.