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Mesoscale and Nanoscale Physics (cond-mat.mes-hall)

Wed, 03 May 2023

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1.Photon emission statistics of a driven microwave cavity

Authors:Pedro Portugal, Fredrik Brange, Kalle S. U. Kansanen, Peter Samuelsson, Christian Flindt

Abstract: Recent experimental advances have made it possible to detect individual quantum jumps in open quantum systems, such as the tunneling of single electrons in nanoscale conductors or the emission of photons from non-classical light sources. Here, we investigate theoretically the statistics of photons emitted from a microwave cavity that is driven resonantly by an external field. We focus on the differences between a parametric and a coherent drive, which either squeezes or displaces the cavity field. We employ a Lindblad master equation dressed with counting fields to obtain the generating function of the photon emission statistics using a theoretical framework based on Gaussian states. We then compare the distribution of photon waiting times for the two drives as well as the $g^{(2)}$-functions of the outgoing light, and we identify important differences between these observables. In the long-time limit, we analyze the factorial cumulants of the photon emission statistics and the large-deviation statistics of the emission currents, which are markedly different for the two drives. Our theoretical framework can readily be extended to more complicated systems, for instance, with several coupled microwave cavities, and our predictions may be tested in future experiments.

2.Topological phase detection through high-harmonic spectroscopy in extended Su-Schrieffer-Heeger chains

Authors:Mohit Lal Bera, Jessica O. de Almeida, Marlena Dziurawiec, Marcin Płodzień, Maciej M. Maśka, Maciej Lewenstein, Tobias Grass, Utso Bhattacharya

Abstract: Su-Schrieffer-Heeger (SSH) chains are paradigmatic examples of 1D topological insulators hosting zero-energy edge modes when the bulk of the system has a non-zero topological winding invariant. Recently, high-harmonic spectroscopy has been suggested as a tool for detecting the topological phase. Specifically, it has been shown that when the SSH chain is coupled to an external laser field of a frequency much smaller than the band gap, the emitted light at harmonic frequencies strongly differs between the trivial and the topological phase. However, it remains unclear whether various non-trivial topological phases -- differing in the number of edge states -- can also be distinguished by the high harmonic generation (HHG). In this paper, we investigate this problem by studying an extended version of the SSH chain with extended-range hoppings, resulting in a topological model with different topological phases. We explicitly show that HHG spectra are a sensitive and suitable tool for distinguishing topological phases when there is more than one topological phase. We also propose a quantitative scheme based on tuning the filling of the system to precisely locate the number of edge modes in each topological phase of this chain.

3.Ultrafast dynamics of bright and dark excitons in monolayer WSe$_2$ and heterobilayer WSe$_2$/MoS$_2$

Authors:Jan Philipp Bange I. Physikalisches Institut, Georg-August-Universität Göttingen, Friedrich-Hund-Platz 1, 37077 Göttingen, Germany, Paul Werner I. Physikalisches Institut, Georg-August-Universität Göttingen, Friedrich-Hund-Platz 1, 37077 Göttingen, Germany, David Schmitt I. Physikalisches Institut, Georg-August-Universität Göttingen, Friedrich-Hund-Platz 1, 37077 Göttingen, Germany, Wiebke Bennecke I. Physikalisches Institut, Georg-August-Universität Göttingen, Friedrich-Hund-Platz 1, 37077 Göttingen, Germany, Giuseppe Meneghini Fachbereich Physik, Philipps-Universität, 35032 Marburg, Germany, AbdulAziz AlMutairi Department of Engineering, University of Cambridge, Cambridge CB3 0FA, U.K, Marco Merboldt I. Physikalisches Institut, Georg-August-Universität Göttingen, Friedrich-Hund-Platz 1, 37077 Göttingen, Germany, Kenji Watanabe Research Center for Electronic and Optical Materials, National Institute for Materials Science, 1-1 Namiki, Tsukuba 305-0044, Japan, Takashi Taniguchi Research Center for Materials Nanoarchitectonics, National Institute for Materials Science, 1-1 Namiki, Tsukuba 305-0044, Japan, Sabine Steil I. Physikalisches Institut, Georg-August-Universität Göttingen, Friedrich-Hund-Platz 1, 37077 Göttingen, Germany, Daniel Steil I. Physikalisches Institut, Georg-August-Universität Göttingen, Friedrich-Hund-Platz 1, 37077 Göttingen, Germany, R. Thomas Weitz I. Physikalisches Institut, Georg-August-Universität Göttingen, Friedrich-Hund-Platz 1, 37077 Göttingen, Germany International Center for Advanced Studies of Energy Conversion, Stephan Hofmann Department of Engineering, University of Cambridge, Cambridge CB3 0FA, U.K, G. S. Matthijs Jansen I. Physikalisches Institut, Georg-August-Universität Göttingen, Friedrich-Hund-Platz 1, 37077 Göttingen, Germany, Samuel Brem Fachbereich Physik, Philipps-Universität, 35032 Marburg, Germany, Ermin Malic Fachbereich Physik, Philipps-Universität, 35032 Marburg, Germany, Marcel Reutzel I. Physikalisches Institut, Georg-August-Universität Göttingen, Friedrich-Hund-Platz 1, 37077 Göttingen, Germany, Stefan Mathias I. Physikalisches Institut, Georg-August-Universität Göttingen, Friedrich-Hund-Platz 1, 37077 Göttingen, Germany International Center for Advanced Studies of Energy Conversion

Abstract: The energy landscape of optical excitations in mono- and few-layer transition metal dichalcogenides (TMDs) is dominated by optically bright and dark excitons. These excitons can be fully localized within a single TMD layer, or the electron- and the hole-component of the exciton can be charge-separated over multiple TMD layers. Such intra- or interlayer excitons have been characterized in detail using all-optical spectroscopies, and, more recently, photoemission spectroscopy. In addition, there are so-called hybrid excitons whose electron- and/or hole-component are delocalized over two or more TMD layers, and therefore provide a promising pathway to mediate charge-transfer processes across the TMD interface. Hence, an in-situ characterization of their energy landscape and dynamics is of vital interest. In this work, using femtosecond momentum microscopy combined with many-particle modeling, we quantitatively compare the dynamics of momentum-indirect intralayer excitons in monolayer WSe$_2$ with the dynamics of momentum-indirect hybrid excitons in heterobilayer WSe$_2$/MoS$_2$, and draw three key conclusions: First, we find that the energy of hybrid excitons is reduced when compared to excitons with pure intralayer character. Second, we show that the momentum-indirect intralayer and hybrid excitons are formed via exciton-phonon scattering from optically excited bright excitons. And third, we demonstrate that the efficiency for phonon absorption and emission processes in the mono- and the heterobilayer is strongly dependent on the energy alignment of the intralayer and hybrid excitons with respect to the optically excited bright exciton. Overall, our work provides microscopic insights into exciton dynamics in TMD mono- and bilayers.

4.Impacts of the half-skyrmion spin topology, spin-orbit torque, and dynamic symmetry breaking on the growth of magnetic stripe domains

Authors:Jeffrey A. Brock, Daan Swinkels, Bert Koopmans, Eric E. Fullerton

Abstract: We have performed an experimental and modeling-based study of the spin-orbit torque-induced growth of magnetic stripe domains in heavy metal/ferromagnet thin-film heterostructures that possess chiral N\'eel-type domain walls due to an interfacial Dzyaloshinskii-Moriya interaction. In agreement with previous reports, the stripe domains stabilized in these systems exhibit a significant transverse growth velocity relative to the applied current axis. This behavior has previously been attributed to the Magnus force-like skyrmion Hall effect of the stripe domain spin topology, which is analogous to that of a half-skyrmion. However, through analytic modeling of the in-plane torques generated by spin-orbit torque, we find that a dynamical reconfiguration of the domain wall magnetization profile is expected to occur - promoting motion with similar directionality and symmetry as the skyrmion Hall effect. These results further highlight the sensitivity of spin-orbit torque to the local orientation of the domain wall magnetization profile and its contribution to domain growth directionality.

5.Thermally-driven Multilevel Non-volatile Memory with Monolayer MoS2 for Neuro-inspired Artificial Learning

Authors:Sameer Kumar Mallik, Roshan Padhan, Mousam Charan Sahu, Suman Roy, Gopal K Pradhan, Prasana Kumar Sahoo, Saroj Prasad Dash, Satyaprakash Sahoo

Abstract: The demands of modern electronic components require advanced computing platforms for efficient information processing to realize in-memory operations with a high density of data storage capabilities towards developing alternatives to von Neumann architectures. Herein, we demonstrate the multifunctionality of monolayer MoS2 mem-transistors which can be used as a high-geared intrinsic transistor at room temperature; however, at a high temperature (>350 K), they exhibit synaptic multi-level memory operations. The temperature-dependent memory mechanism is governed by interfacial physics, which solely depends on the gate field modulated ion dynamics and charge transfer at the MoS2/dielectric interface. We have proposed a non-volatile memory application using a single FET device where thermal energy can be ventured to aid the memory functions with multi-level (3-bit) storage capabilities. Furthermore, our devices exhibit linear and symmetry in conductance weight updates when subjected to electrical potentiation and depression. This feature has enabled us to attain a high classification accuracy while training and testing the Modified National Institute of Standards and Technology datasets through artificial neural network simulation. This work paves the way for new avenues in 2D semiconductors toward reliable data processing and storage with high-packing density arrays for brain-inspired artificial learning.

6.Antiferromagnetic Bloch line driven by spin current as room-temperature analog of a fluxon in a long Josephson junction

Authors:R. V. Ovcharov, B. A. Ivanov, J. Åkerman, R. S. Khymyn

Abstract: Antiferromagnets (AFMs) are promising materials for future high-frequency field-free spintronic applications. Self-localized spin structures can enhance their capabilities and introduce new functionalities to AFM-based devices. Here we consider a domain wall (DW), a topological soliton that bridges a connection between two ground states, similar to a Josephson junction (JJ) link between two superconductors. We demonstrate the similarities between DWs in bi-axial AFM with easy-axis primary anisotropy, driven by a spin current, and long Josephson junctions (LJJs). We found that the Bloch line (BL) in DWs resembles the fluxon state of JJs, creating a close analogy between the two systems. We propose a scheme that allows us to create, move, read, and delete such BLs. This transmission line operates at room temperature and can be dynamically reconfigured in contrast to superconductors. Results of a developed model were confirmed by micromagnetic simulations for Cr$_2$O$_3$ and DyFeO$_3$, i.e., correspondingly with weak and strong in-plane anisotropy. Overall, the proposed scheme has significant potential for use in magnetic memory and logic devices.