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Mesoscale and Nanoscale Physics (cond-mat.mes-hall)

Mon, 26 Jun 2023

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1.Controllable magnetic domains in twisted trilayer magnets

Authors:Kyoung-Min Kim, Moon Jip Park

Abstract: The use of moir\'e patterns to manipulate two-dimensional materials has facilitated new possibilities for controlling material properties. The moir\'e patterns in the two-dimensional magnets can cause peculiar spin texture, as shown by previous studies focused on twisted bilayer systems. In our study, we develop a theoretical model to investigate the magnetic structure of twisted trilayer magnets. Unlike the twisted bilayer, the twisted trilayer magnet has four different local stacking structures distinguished by the interlayer couplings between the three layers. Our results show that the complex interlayer coupling effects in the moir\'e superlattice can lead to the stabilization of rich magnetic domain structures; these structures can be significantly manipulated by adjusting the twist angle. Additionally, external magnetic fields can easily manipulate these domain structures, indicating potential applications in spintronics devices.

2.Eigenvalues of regular symmetric Hall-plates

Authors:Udo Ausserlechner

Abstract: I discuss uniform, isotropic, plane, singly connected, electrically linear, regular symmetric Hall-plates with an arbitrary number of N peripheral contacts exposed to a uniform perpendicular magnetic field of arbitrary strength. In practice, the regular symmetry is the most common one. If the Hall-plates are mapped conformally to the unit disk, regular symmetry means that all contacts are equally large and all contacts spacings are equally large, yet the contacts spacings may have a different size than the contacts. Such Hall-plates do not change when they are rotated by 360{\deg}/N. Their indefinite conductance matrices are circulant matrices, whose complex eigenvalues are computable in closed form. These eigenvalues are used to discuss the Hall-output voltage, the maximum noise-efficiency, and Van-der-Pauw's method for measuring sheet resistances. For practical use, I report simple approximations for Hall-plates with four contacts and 90{\deg} symmetry with popular shapes like disks, rectangles, octagons, squares, and Greek crosses with and without rounded corners.

3.Phenomenon of multiple reentrant localization in a double-stranded helix with transverse electric field

Authors:Sudin Ganguly, Suparna Sarkar, Kallol Mondal, Santanu K. Maiti

Abstract: The present work explores the potential for observing multiple reentrant localization behavior in a double-stranded helical (DSH) system, extending beyond the conventional nearest-neighbor hopping interaction. The DSH system is considered to have hopping dimerization in each strand, while also being subjected to a transverse electric field. The inclusion of an electric field serves the dual purpose of inducing quasiperiodic disorder and strand-wise staggered site energies. Two reentrant localization regions are identified: one exhibiting true extended behavior in the thermodynamic limit, while the second region shows quasi-extended characteristics with partial spreading within the helix. The DSH system exhibits three distinct single-particle mobility edges linked to localization transitions present in the system. The analysis in this study involves examining various parameters such as the single-particle energy spectrum, inverse participation ratio, local probability amplitude, and more. Our proposal, combining achievable hopping dimerization and induced correlated disorder, presents a unique opportunity to study phenomenon of reentrant localization, generating significant research interest.

4.Electron Teleportation via Multiple Majorana Bound States in a Superconductor Island

Authors:Zhen-Tao Zhang, Bao-Long Liang, Zhen-Shan Yang

Abstract: Electron teleportation via two separate Majorana bound states(MBSs) is a manifestation of the non-locality of MBSs. A superconductor may host multiple separate or partial overlapping MBSs, and it is difficult to distinguish them. Here, we have studied the electron teleportation between two quantum dots via multiple MBSs in a superconductor island, two of which couple with the quantum dots. We find that in the absence of Majorana coupling, both elastic and inelastic electron transfers are allowed for specific system settings, and the extent to which the island state is changed after the teleportation relies on the initial state of the MBSs. In the presence of Majorana couplings, the elastic and inelastic teleportations are selective according to which pair of MBSs are coupled. Meanwhile, the cotuneling processes are distinct for different MBSs coupling types. In addition, we have investigated the effect of the asymmetry of the tunnelings to quantum dots on the transport. Our findings are meaningful for resolving transport signatures induced by topological MBSs and that stems from nontopological quasiparticle.

5.Elucidating Interfacial Dynamics of Ti-Al Systems Using Molecular Dynamics Simulation and Markov State Modeling

Authors:Tianjiao Li, Chenxi Tian, Atieh Moridi, Jingjie Yeo

Abstract: Due to their remarkable mechanical and chemical properties, Ti-Al based materials are attracting considerable interest in numerous fields of engineering, such as automotive, aerospace, and defense. With their low density, high strength, and resistance to corrosion and oxidation, these intermetallic alloys and compound metal-metallic composites have found diverse applications. The present study delves into the interfacial dynamics of these Ti-Al systems, particularly focusing on the behavior of Ti and Al atoms in the presence of TiAl$_3$ grain boundaries under experimental heat treatment conditions. Using a combination of Molecular Dynamics and Markov State Model analyses, we scrutinize the kinetic processes involved in the formation of TiAl$_3$. The Molecular Dynamics simulation indicates that at the early stage of heat treatment, the predominating process is the diffusion of Al atoms towards the Ti surface through the TiAl$_3$ grain boundaries. The Markov State Modeling identifies three distinct dynamic states of Al atoms within the Ti/Al mixture that forms during the process, each exhibiting a unique spatial distribution. Using transition timescales as a qualitative measure of the rapidness of the dynamics, it is observed that the Al dynamics is significantly less rapid near the Ti surface compared to the Al surface. Put together, the results offer a comprehensive understanding of the interfacial dynamics and reveals a three-stage diffusion mechanism. The process initiates with the premelting of Al, proceeds with the prevalent diffusion of Al atoms towards the Ti surface, and eventually ceases as the Ti concentration within the mixture progressively increases. The insights gained from this study could contribute significantly to the control and optimization of manufacturing processes for these high-performing Ti-Al based materials.

6.Photon Correlations in Colloidal Quantum Dot Molecules Controlled by the Neck Barrier

Authors:Somnath Koley, Jiabin Cui, Yossef. E. Panfil, Yonatan Ossia, Adar Levi, Einav Scharf, Lior Verbitsky, Uri Banin

Abstract: We investigate the charge re-distribution upon optical excitation of various necked homodimer CQDMs using single particle emission spectroscopy. By tuning the hybridization of the electron wavefunction at a fixed center-to-center distance through controlling the neck girth, we reveal two coupling limits. On one hand a connected-but-confined situation where neighbouring CQDs are weakly fused to each other manifesting a weak coupling regime, and on the other hand, a connected-and-delocalized situation, where the neck is filled beyond the facet size leading to a rod-like architecture manifesting strong-coupling. Either coupling regimes entrust distinct optical signatures clearly resolved at room temperature in terms of photoluminescence quantum yield, intensity time traces, lifetimes, and spectra of the neutral-exciton, charged-exciton, and biexciton states. The interplay between the radiative and non-radiative Auger decays of these states, turns emitted photons from the CQDMs in the weak-coupling regime highly bunched unlike CQD monomers, while the antibunching is regained at the strong-coupling regime. This behavior correlates with the hybridization energy being smaller than the thermal energy (kT approx. 25meV) at the weak-coupling limit (delta E approax.5-10meV), leading to exciton localization suppressing Auger decay. In the neck-filled architectures, the larger hybridization energy (delta E approx.20-30meV) leads to exciton delocalization while activating the fast charged and multi-exciton Auger decay processes. This work sets an analogy for the artificial molecule CQDMs with regular molecules, where the two distinct regimes of weak- and strong-coupling correspond to ionic- or covalent- type bonding, respectively.

7.Zn-doped P-type InAs Nanocrystal Quantum Dots

Authors:Lior Asor, Jing Liu, Shuting Xiang, Nir Tessler, Anatoly I. Frenkel, Uri Banin

Abstract: Doped heavy metal-free III-V semiconductor nanocrystal quantum dots are of great interest both from the fundamental aspects of doping in highly confined structures, and from the applicative side of utilizing such building blocks in the fabrication of p-n homojunction devices. InAs nanocrystals, that are of particular relevance for short wave IR detection and emission applications, manifest heavy n-type character poising a challenge for their transition to p-type behavior. We present p-type doping of InAs nanocrystals with Zn-enabling control over the charge carrier type in InAs QDs field effect transistors. The post-synthesis doping reaction mechanism is studied for Zn precursors with varying reactivity. Successful p-type doping was achieved by the more reactive precursor, diethylzinc. Substitutional doping by Zn2+ replacing In3+ is established by X-ray absorption spectroscopy analysis. Furthermore, enhanced near IR photoluminescence is observed due to surface passivation by Zn as indicated from elemental mapping utilizing high resolution electron microscopy corroborated by X-ray photoelectron spectroscopy study. The demonstrated ability to control the carrier type, along with the improved emission characteristics, paves the way towards fabrication of optoelectronic devices active in the short wave IR region utilizing heavy-metal free nanocrystal building blocks.

8.Noise and fluctuations in nanoscale gas flow

Authors:J. Dastoor, D. M. Willerton, W. Reisner, G. Gervais

Abstract: We theoretically calculate the fundamental noise that is present in gaseous (dilute fluid) flow in channels in the classical and degenerate quantum regime, where the Fermi-Dirac and Bose- Einstein distribution must be considered. Results for both regimes are analogous to their electrical counterparts. The quantum noise is calculated for a two terminal system and is a complicated function of the thermal and shot noise with the thermal noise dominating when $2k_BT >> m\Delta P$ and vice versa. The cumulant generating function for mass flow, which generates all the higher order statistics related to our mass flow distribution, is also derived and is used to find an expression for the third cumulant of flow across a fluidic channel.

9.Non-Hermitian chiral anomalies in interacting systems

Authors:Sharareh Sayyad

Abstract: The emergence of chiral anomaly entails various fascinating phenomena such as anomalous quantum Hall effect and chiral magnetic effect in different branches of (non-)Hermitian physics. While in the single-particle picture, anomalous currents merely appear due to the coupling of massless particles with background fields, many-body interactions can also be responsible for anomalous transport in interacting systems. In this Letter, we study anomalous chiral currents in systems where interacting massless fermions with complex Fermi velocities are coupled to complex gauge fields. Our results reveal that incorporating non-Hermiticity and many-body interactions gives rise to additional terms in anomalous relations beyond their Hermitian counterparts. We further present that many-body corrections in the subsequent non-Hermitian chiral magnetic field or anomalous Hall effect are nonvanishing in nonequilibrium or inhomogeneous systems. Our results advance efforts in understanding the anomalous transport in interacting non-Hermitian systems.

10.An open-source robust machine learning platform for real-time detection and classification of 2D material flakes

Authors:Jan-Lucas Uslu, Taoufiq Ouaj, David Tebbe, Jo Henri Bertram, Marc Schütte, Kenji Watanabe, Takashi Taniguchi, Bernd Beschoten, Lutz Waldecker, Christoph Stampfer

Abstract: The most widely used method for obtaining high-quality two-dimensional materials is through mechanical exfoliation of bulk crystals. Manual identification of suitable flakes from the resulting random distribution of crystal thicknesses and sizes on a substrate is a time-consuming, tedious task. Here, we present a platform for fully automated scanning, detection, and classification of two-dimensional materials, the source code of which we make openly available. Our platform is designed to be accurate, reliable, fast, and versatile in integrating new materials, making it suitable for everyday laboratory work. The implementation allows a fully automized scanning and analysis of wafers with an average inference time of 100 ms for images of 2.3 Mpixels. The developed detection algorithm is based on a combination of the flakes' optical contrast toward the substrate and their geometric shape. We demonstrate that it is able to detect the majority of exfoliated flakes of various materials, with an average recall (AR50) between 66\% and 92\%. We also show that the algorithm can be trained with as few as five flakes of a given material, which we demonstrate for the examples of few-layer graphene, WSe$_2$, CrI$_3$, 1T-TaS$_2$ and hBN. Our platform has been tested over a two-year period, during which more than 10$^6$ images of multiple different materials were acquired by over 30 individual researchers.