Mesoscale and Nanoscale Physics (cond-mat.mes-hall)

Abstract: Harnessing electronic excitations involving coherent coupling to bosonic modes is essential for the design and control of emergent phenomena in quantum materials [1]. In situations where charge carriers induce a lattice distortion due to the electron-phonon interaction, the conducting states get "dressed". This leads to the formation of polaronic quasiparticles that dramatically impact charge transport, surface reactivity, thermoelectric and optical properties, as observed in a variety of crystals and interfaces composed of polar materials [2-6]. Similarly, when oscillations of the charge density couple to conduction electrons the more elusive plasmon polaron emerges [7], which has been detected in electron-doped semiconductors [8-10]. However, the exploration of polaronic effects on low energy excitations is still in its infancy in two-dimensional (2D) materials. Here, we present the discovery of an interlayer plasmon polaron in heterostructures composed of graphene on top of SL WS$_2$. By using micro-focused angle-resolved photoemission spectroscopy (microARPES) during in situ doping of the top graphene layer, we observe a strong quasiparticle peak accompanied by several carrier density-dependent shake-off replicas around the SL WS$_2$ conduction band minimum (CBM). Our results are explained by an effective many-body model in terms of a coupling between SL WS$_2$ conduction electrons and graphene plasmon modes. It is important to take into account the presence of such interlayer collective modes, as they have profound consequences for the electronic and optical properties of heterostructures that are routinely explored in many device architectures involving 2D transition metal dichalcogenides (TMDs) [11-15].

Abstract: An electrical current that flows across individual atoms or molecules can generate exotic quantum-based behavior, from memristive effects to Coulomb blockade and the promotion of quantum excited states. These fundamental effects typically appear one at a time in model junctions built using atomic tip or lateral techniques. So far, however, a viable industrial pathway for such discrete state devices has been lacking. Here, we demonstrate that a commercialized device platform can serve as this industrial pathway for quantum technologies. We have studied magnetic tunnel junctions with a MgO barrier containing C atoms. The paramagnetic localized electrons due to individual C atoms generate parallel nanotransport paths across the micronic device as deduced from magnetotransport experiments. Coulomb blockade effects linked to tunnelling magnetoresistance peaks can be electrically controlled, leading to a persistent memory effect. Our results position MgO tunneling spintronics as a promising platform to industrially implement quantum technologies.

Abstract: Ultrafast light-matter interaction has emerged as a powerful tool to control and probe the macroscopic properties of functional materials, especially two-dimensional transition metal dichalcogenides which can form different structural phases with distinct physical properties. However, it is often difficult to accurately determine the transient optical constants. In this work, we developed a near-infrared pump - terahertz to midinfrared (12-22 THz) probe system in transmission geometry to measure the transient optical conductivity in 2H-MoTe2 layered material. By performing separate measurements on bulk and thin-film samples, we are able to overcome issues related to nonuniform substrate thickness and penetration depth mismatch and to extract the transient optical constants reliably. Our results show that photoexcitation at 690 nm induces a transient insulator-metal transition, while photoexcitation at 2 um has a much smaller effect due to the photon energy being smaller than the band gap of the material. Combining this with a single-color pump-probe measurement, we show that the transient response evolves towards 1T' phase at higher flunece. Our work provides a comprehensive understanding of the photoinduced phase transition in the 2H-MoTe2 system.

Abstract: Generalized multifractality characterizes system size dependence of pure scaling local observables at Anderson transitions in all ten symmetry classes of disordered systems. Recently, the concept of generalized multifractality has been extended to boundaries of critical disordered noninteracting systems. Here we study the generalized boundary multifractality in the presence of electron-electron interaction, focusing on the spin quantum Hall symmetry class (class C). Employing the two-loop renormalization group analysis within Finkel'stein nonlinear sigma model we compute the anomalous dimensions of the pure scaling operators located at the boundary of the system. We find that generalized boundary multifractal exponents are twice larger than their bulk counterparts. Exact symmetry relations between generalized boundary multifractal exponents in the case of noninteracting systems are explicitly broken by the interaction.

Abstract: Nontrivial bulk topological invariants of quantum materials can leave their signatures on charge, thermal and spin transports. In two dimensions, their imprints can be experimentally measured from well-developed multi-terminal Hall bar arrangements. Here, we numerically compute the low temperature ($T$) thermal ($\kappa_{xy}$) and zero temperature spin ($\sigma^{sp}_{xy}$) Hall conductivities, and longitudinal thermal conductance ($G^{th}_{xx}$) of various paradigmatic two-dimensional fully gapped topological superconductors, belonging to distinct Altland-Zirnbauer symmetry classes, namely $p+ip$ (class D), $d+id$ (class C) and $p \pm ip$ (class DIII) paired states, in mesoscopic six-terminal Hall bar setups from the scattering matrix formalism using Kwant. In both clean and weak disorder limits, the time-reversal symmetry breaking $p+ip$ and $d+id$ pairings show half-quantized and quantized $\kappa_{xy}$ [in units of $\kappa_0=\pi^2 k^2_B T/(3h)$], respectively, while the latter one in addition accommodates a quantized $\sigma^{sp}_{xy}$ [in units of $\sigma^{sp}_0=\hbar/(8 \pi)$]. By contrast, the time-reversal invariant $p \pm ip$ pairing only displays a quantized $G^{th}_{xx}$ at low $T$ up to a moderate strength of disorder. In the strong disorder regime, all these topological responses ($\kappa_{xy}$, $\sigma^{sp}_{xy}$ and $G^{th}_{xx}$) vanish. Possible material platforms hosting such paired states and manifesting these robust topological thermal and spin responses are highlighted.