Mesoscale and Nanoscale Physics (cond-mat.mes-hall)

Abstract: The periodic Toda lattice can be solved by exploiting the spectral properties of the Lax operator, where boundary states play an important role. We show that such boundary states have a topological origin similar to the edge states in topological insulators, and consequently, bulk wave functions of the Lax operator yield nontrivial Chern numbers. This implies that the periodic Toda lattice belongs to the same topological class as the Thouless pump. We demonstrate that the cnoidal wave of the Toda lattice shows Chern number $-1$ per period.

Abstract: Semiconductor quantum dot molecules are considered as promising candidates for quantum technological applications due to their wide tunability of optical properties and coverage of different energy scales associated with charge and spin physics. While previous works have studied the tunnel-coupling of the different excitonic charge complexes shared by the two quantum dots by conventional optical spectroscopy, we here report on the first demonstration of a coherently controlled inter-dot tunnel-coupling focusing on the quantum coherence of the optically active trion transitions. We employ ultrafast four-wave mixing spectroscopy to resonantly generate a quantum coherence in one trion complex, transfer it to and probe it in another trion configuration. With the help of theoretical modelling on different levels of complexity we give an instructive explanation of the underlying coupling mechanism and dynamical processes.

Abstract: Cubic chiral magnets exhibit a remarkable diversity of two-dimensional topological magnetic textures, including skyrmions. However, the experimental confirmation of topological states localized in all three spatial dimensions remains challenging. In this paper, we investigate a three-dimensional topological state called a heliknoton, which is a hopfion embedded into a helix or conic background. We explore the range of parameters at which the heliknoton can be stabilized under realistic conditions using micromagnetic modeling, harmonic transition state theory, and stochastic spin dynamics simulations. We present theoretical Lorentz TEM images of the heliknoton, which can be used for experimental comparison. Additionally, we discuss the stability of the heliknoton at finite temperatures and the mechanism of its collapse. Our study offers a pathway for future experimental investigations of three-dimensional topological solitons in magnetic crystals.

Abstract: PbTe nanowires coupled to a superconductor have recently been proposed as a potential Majorana platform. The hallmark of the one-dimensional nature of ballistic nanowires is their quantized conductance. Here, we report the observation of conductance plateaus at multiples of the quantized value $2e^2/h$ in PbTe nanowires at finite magnetic fields. The quantized plateaus, as a function of source-drain bias and magnetic field, allow for the extraction of the Land\'e $g$-factor, sub-band spacing and effective mass. The coefficient of 2 in the plateau conductance indicates the presence of valley degeneracy arising from the crystal orientation of the nanowires, which are grown on a (001) substrate. Occasionally, this degeneracy can be lifted by a gate voltage that breaks the mirror symmetry. Our results demonstrate the one-dimensionality of PbTe nanowires and fulfill one of the necessary conditions for the realization of Majorana zero modes.

Abstract: One of the key challenges for spintronic and novel quantum technologies is to achieve active control of the spin angular momentum of electrons in nanoscale materials on ultrafast, femtosecond timescales. While conventional ferromagnetic materials and materials supporting spin texture suffer both from conceptional limitations in miniaturization and in efficiency of optical and electronic manipulation, non-magnetic centrosymmetric layered materials with hidden spin polarization may offer an alternative pathway to manipulate the spin degree of freedom by external stimuli. Here we demonstrate a novel approach to generate transient spin polarization on a femtosecond timescale in the otherwise spin-unpolarized band structure of the centrosymmetric 2H-stacked group VI transition metal dichalcogenide WSe$_{2}$. Using ultrafast optical excitation of a fullerene layer grown on top of WSe$_{2}$, we trigger an ultrafast interlayer electron transfer from the fullerene layer into the WSe$_{2}$ crystal. The resulting transient charging of the C$_{60}$/WSe$_{2}$ interface leads to a substantial interfacial electric field that by means of spin-layer-valley locking ultimately creates ultrafast spin polarization without the need of an external magnetic field. Our findings hence open a novel pathway for optically engineering spin functionalities such as the sub-picosecond generation and manipulation of ultrafast spin currents in 2D heterostructures.

Abstract: We investigate the decay of spatial correlations of $\mathcal{PT}$-symmetric non-Hermitian one-dimensional models that host higher-order exceptional points. Beyond a certain correlation length, they develop anomalous power-law behavior that indicates strong suppression of correlations in the non-Hermitian setups as compared to the Hermitian ones. The correlation length is also reflected in the entanglement entropy where it marks a change from logarithmic growth at short distance to a constant value at large distance, characteristic of an insulator, despite the spectrum being gapless. Two different families of models are investigated, both having a similar spectrum constrained by particle-hole symmetry. The first model offers an experimentally attractive way to generate arbitrary higher-order exceptional points and represents a non-Hermitian extension of the Dirac Hamiltonian for general spin. At the critical point it displays a decay of the correlations $\sim 1/x^2$ and $1/x^3$ irrespective of the order of the exceptional point. The second model is constructed using unidirectional hopping and display enhanced suppression of correlations $\sim 1/x^a$, $a\ge 2$ with a power law that depends on the order of the exceptional point.

Abstract: High-quality free-standing InAs nanosheets are emerging layered semiconductor materials with potentials in designing planar Josephson junction devices for novel physics studies due to their unique properties including strong spin-orbit couplings, large Land\'e g-factors and the two dimensional nature. Here, we report an experimental study of proximity induced superconductivity in planar Josephson junction devices made from free-standing InAs nanosheets. The nanosheets are grown by molecular beam epitaxy and the Josephson junction devices are fabricated by directly contacting the nanosheets with superconductor Al electrodes. The fabricated devices are explored by low-temperature carrier transport measurements. The measurements show that the devices exhibit a gate-tunable supercurrent, multiple Andreev reflections, and a good quality superconductor-semiconductor interface. The superconducting characteristics of the Josephson junctions are investigated at different magnetic fields and temperatures, and are analyzed based on the Bardeen-Cooper-Schrieffer (BCS) theory. The measurements of ac Josephson effect are also conducted under microwave radiations with different radiation powers and frequencies, and integer Shapiro steps are observed. Our work demonstrates that InAs nanosheet based hybrid devices are desired systems for investigating forefront physics, such as the two-dimensional topological superconductivity.

Abstract: We report a study on the relationship between structure and electron transport properties of nanoscale graphene/pentacene interfaces. We fabricated graphene/pentacene interfaces from 10-30 nm thick needle-like pentacene nanostructures down to two-three layers (2L-3L) dendritic pentacene islands, and we measured their electron transport properties by conductive atomic force microscopy (C-AFM). The energy barrier at the interfaces, i.e. the energy position of the pentacene highest occupied molecular orbital (HOMO) with respect to the Fermi energy of the graphene and the C-AFM metal tip, are determined and discussed with the appropriate electron transport model (double Schottky diode model and Landauer-Buttiker model, respectively) taking into account the voltage-dependent charge doping of graphene. In both types of samples, the energy barrier at the graphene/pentacene interface is slightly larger than that at the pentacene/metal tip interface, resulting in 0.47-0.55 eV and 0.21-0.34 eV, respectively, for the 10-30 nm thick needle-like pentacene islands, and in 0.92-1.44 eV and 0.67-1.05 eV, respectively, for the 2L-3L thick dendritic pentacene nanostructures. We attribute this difference to the molecular organization details of the pentacene/graphene heterostructures, with pentacene molecules lying flat on the graphene in the needle-like pentacene nansotructures, while standing upright in 2L-3L dendritic islands, as observed from Raman spectroscopy.

Abstract: We examine the transmissions in gapped graphene through a combination of double barriers tilting and time-oscillating potential. The latter introduces extra sidebands to the transmission probability, which occur at energy levels determined by the frequency and incident energy. The sidebands are generated as a result of the absorption or emission of photons yielded from the oscillating potential. Our results indicate that transmission probabilities in gapped graphene can be manipulated by regulating the incident energy, the oscillating potential, or the distance between two barriers and their heights. It has been observed that the transmissions may be impeded or prevented by tuning the gap.

Abstract: The quasicharge superconducting qubit realizes the dual of the transmon and shows strong robustness to flux and charge fluctuations thanks to a very large inductance closed on a Josephson junction. At the same time, a weak anharmonicity of the spectrum is inherited from the parent transmon, that introduces leakage errors and is prone to frequency crowding in multi-qubit setups. We propose a novel design that employs a quartic superinductor and confers a good degree of anharmonicity to the spectrum. The quartic regime is achieved through a properly designed chain of Josephson junction loops that avoids strong quantum fluctuations without introducing a severe dependence on the external flux.

Abstract: Photocurrent acts as one of measurable responses of material to light, which has proved itself to be crucial for sensing and energy harvesting. Topological semimetals with gapless energy dispersion and abundant topological surface and bulk states exhibit exotic photocurrent responses, such as novel quantized circular photogalvanic effect observed in Weyl semimetals. Here we find that for a topological nodal-line semimetal (NLSM) with nodal ring bulk states and drumhead surface states (DSS), a significant photocurrent can be produced by an electromagnetic (EM) wave by means of the quantum Hall effect. The Hall current is enabled by electron transfer between Landau levels (LLs) and triggered by both the electric field and magnetic field components of an EM wave. This Hall current is physically connected to an unusually large quantum-Hall conductivity of the zeroth LLs resulting from quantized DSS. These LLs are found to be highly degenerate due to the unique band-folding effect associated with magnetic-field-induced expansion of a unit cell. Furthermore, we observe that the Hall current induced solely by an in-plane linearly-polarized EM wave becomes a quantized entity which allows for possible direct measurement of the DSS density in a topological NLSM. This work paves a way toward designing high-magnetic-field-sensitivity detection devices for industrial and space applications, such as the development of self-detection of current-surge-induced overheating in electronic devices and accurate Earth's magnetic-anomaly maps for guiding a self-navigating drone or an aircraft.

Abstract: We consider non-dissipative drag between Bose-condensed exciton polaritons in optical microcavity and embedded superconductors. This effect consists in induction of a non-dissipative electric current in the superconductor by motion of polariton Bose condensate due to electron-polariton interaction, or vice versa. Using many-body theory, we calculate the drag density, characterizing magnitude of this effect, with taking into account dynamical screening of the interaction. Hoping to diminish the interaction screening and microcavity photon absorption, we consider atomically-thin superconductors (both conventional s-wave and copper-oxide d-wave) of planar and nanoribbon shapes. Our estimates show that in realistic conditions the drag effect could be rather weak but observable in accurate experiments in the case of dipolar interlayer excitons in transition metal dichalcogenide bilayers. Use of spatially direct excitons, semiconductor quantum wells as the host for excitons, or thin films of bulk metallic superconductors considerably lowers the drag density.